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A common molecular design paradigm for optical power limiting (OPL) applications is to introduce heavy atoms that promote intersystem crossing and triplet excited states. In order to investigate this effect, three multi-branched fluorene molecules were prepared where the central moiety was either an organic benzene unit, para-dibromobenzene, or a platinum(II)-alkynyl unit. All three molecules show

Lead-free halide double perovskites have gathered wide scientific interest since they are environmentally friendly and stable. However, compared to the lead perovskites, their optoelectronic properties are compromised. Herein we report a series of bulk lead-free mixed Bi-In halide double perovskites: Cs2AgBi1−xInxCl6 (0

Background: Social and biological circumstances at birth are established predictors of adult socioeconomic position (SEP). This study aims to assess the trends in these associations across two generations and examine the effects of parental early-life characteristics on descendants' adult SEP. Methods: We studied men and women born in the Uppsala University Hospital 1915-1929 (G1) and their offspr

In this work, we explored the photoinduced charge carriers dynamics rationalizing the photocatalytic oxidation of NO over N-doped Bi2O2CO3/graphene quantum dots composites(N-BOC/GQDs) via time-resolved photoluminescence (TRPL). Under visible light illumination, only GQDs can be photoexcited and inject electrons to N-BOC within 0.5 ns. Under UV light irradiation, the interfacial Z-scheme heterojunc

The gain and loss of aromaticity plays a key role in organic chemistry and in the prediction of rate‐determining steps. Herein, we explore the concept of aromaticity in photoisomerization reactions. Benzannulated derivatives of the dihydroazulene‐vinylheptafulvene (DHA‐VHF) photoswitch were investigated using transient absorption spectroscopy and time‐dependent density functional theory to elucida

Colloidal all-inorganic perovskite nanocrystals have gained significant attention as a promising material for both fundamental and applied research due to their excellent emission properties. However, reported photoluminescence quantum yields (PL QYs) of blue-emitting perovskite nanocrystals are rather low, mostly due to the fact that the high energy excitons for such wide bandgap materials are e

Floder och åar är viktiga källor för järn och andra näringsämnen till Östersjön. De senaste decennierna har järnkoncentrationen i svenska och finska åar ökat kraftigt, vilket skulle kunna leda till en ökad transport av järn till Östersjön. Vilken effekt detta kan ha för Östersjön beror på vad som händer med järnet när det möter det salta vattnet i Östersjön. Järn transporteras huvudsakligen i formRivers have traditionally not been considered important sources of bioavailable iron (Fe) to the marine waters, since most Fe is lost by salinity-induced aggregation and sedimentation during estuarine mixing. However, recent studies from boreal rivers found a remarkably high Fe stability, probably due to the interaction with organic matter. Recent studies have suggested that Fe speciation is a key

Background: Previous studies from our and other centers on young patients with type 1 diabetes (T1D) have indicated pro-atherosclerotic changes in the carotid arteries and in the lipid and systemic inflammatory profiles without a clear relationship between these changes and the hyperglycemic control. We have also earlier found in these patients a certain HLA-related genetic susceptibility to adver

All-inorganic CsPbBr3 perovskite colloidal quantum dots have recently emerged as a promising material for a variety of optoelectronic applications, among others for multiphoton-pumped lasing. Nevertheless, high irradiance levels are generally required for such multiphoton processes. One strategy to enhance the multiphoton absorption is taking advantage of high local light intensities using photoni

Choice blindness is a cognitive phenomenon describing that when people receive false feedback about a choice they just made, they often accept the outcome as their own. Little is known about what predisposes people to correct manipulations they are subjected to in choice blindness studies. In this study, 118 participants answered a political attitude survey and were then asked to explain some of t

IMPORTANCE Heart failure (HF) aggregates in families, but the heritability of HF has not been determined. Discerning the genetic and environmental contributions to HF risk is important to further helping to identify individuals at risk. Adoption studies may establish the genetic contribution to HF. OBJECTIVE This nationwide adoption study aimed to determine the heritability of HF. DESIGN, SETTING,

Today's IT organizations must ensure that IT services are aligned to business needs and actively support ongoing business processes. This means that internal IT service management processes are under constant improvement. However, to be able to know if the IT service provision develops in the right direction, there is a need to perform some kind of self-assessment of IT process maturity. In this p

In this paper, we linear quadratic team decision problems, where a team of agents minimizes a convex quadratic cost function over T time steps subject to possibly distinct linear measurements of the state of nature. We assume that the state of nature is a Gaussian random variable and that the agents do not know the cost function nor the linear functions mapping the state of nature to their measure

We study network SIR (Susceptible - Infected - Recovered) epidemic models in the case of two interacting populations. We analyze the dynamics behavior of the fractions of infected individuals in the two populations. In contrast to the classical scalar SIR epidemic model, where the fraction of infected individuals is known to have an unimodal behavior (either decreasing throughout time or initially

Faults and errors are common in the execution of digital controllers on top of embedded hardware. Researchers from the embedded system domain devised models to understand and bound the occurrence of these faults. Using these models, control researchers have demonstrated robustness properties of control systems, and of their corresponding digital implementations. In this paper, we build a framework

System level synthesis is a promising approach that formulates structured optimal controller synthesis problems as convex problems. This work solves the distributed linear-quadratic regulator problem under communication constraints directly in infinite-dimensional space, without the finite-impulse response relaxation common in related work. Our method can also be used to construct optimal distribu

Social influence is largely recognized as a key factor in opinion formation processes. Recently, the role of external forces in inducing opinion displacement and polarization in social networks has attracted significant attention. This is in particular motivated by the necessity to understand and possibly prevent interference phenomena during political campaigns and elections. In this paper, we fo

We present a new, scalable alternative to the structured singular value, which we call v, provide a convex upper bound, study their properties and compare them to l1 robust control. The analysis relies on a novel result on the relationship between robust control of dynamical systems and non-negative constant matrices.

Pregnancy-related factors are important for short- and long-term health in mothers and offspring. The nationwide population-based Swedish Medical Birth Register (MBR) was established in 1973. The present study describes the content and quality of the MBR, using original MBR data, Swedish-language and international publications based on the MBR. The MBR includes around 98% of all births in Sweden.

2D Ruddlesden–Popper (RP) perovskite solar cells have manifested superior operation durability yet inferior charge transport compared to their 3D counterparts. Integrating 3D phases with 2D RP perovskites presents a compromise to maintain respective advantages of both components. Here, the spontaneous generation of 3D phases embedded in 2D perovskite matrix is demonstrated at room temperature via