Exploring Time-Domain Femtosecond Rotational Coherent Raman Scattering for Diagnostics
The diagnostic potential of femtosecond (fs) rotational coherent Raman scattering (RCRS) in the time domain is initially investigated. While RCRS concepts in the spectral domain obtain species selectivity and temperature sensitivity by resolving the spectral shape, mainly reflecting the Boltzmann-distributed, rotational populations of the Raman-active molecules present, the current time-domain fs-
